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Room-Temperature Electrically Driven Tamm-Plasmon Exciton-Polariton LEDs Incorporating Monolayer Perovskite Quantum Dots

  • Meng Cheng Yen
  • , Wei Jie Hong
  • , Hsu Cheng Hsu
  • , Yuto Kajino
  • , Kaoru Tamada*
  • , Gong Ru Lin*
  • , Jinn Kong Sheu*
  • , Ya Ju Lee*
  • *此作品的通信作者

研究成果: 雜誌貢獻期刊論文同行評審

摘要

Electrically driven exciton-polaritons in halide perovskites present a viable route toward room-temperature coherent light sources and polaritonic circuitry, yet experimental realizations remain limited. Here, we demonstrate a room-temperature, electrically driven exciton-polariton light-emitting diode (LED) by embedding a single monolayer of all-inorganic perovskite quantum dots (CsPbBr3 QDs) into a Tamm-plasmon (TP) microcavity comprising a distributed Bragg reflector (DBR) and a silver mirror. The subwavelength QD monolayer simultaneously provides strong exciton oscillator strength and reduces optical mode volume, yielding a large Rabi splitting of (Formula presented.). Time-resolved photoluminescence (PL) reveals a Purcell factor of (Formula presented.), evidencing accelerated radiative recombination and strengthened light-matter coupling. Under optical excitation, an accumulation of polariton population near the lower polariton branch minimum is observed, whereas momentum-resolved electroluminescence (EL) reveals a persistent polariton bottleneck effect under electrical injection. These results establish a scalable, fabrication-compatible platform for electrically driven polaritonic light sources at room temperature, advancing the development of integrated quantum photonic and optoelectronic technologies.

原文英語
文章編號e02503
期刊Laser and Photonics Reviews
20
發行號8
DOIs
出版狀態已發佈 - 2026 4月 17
對外發佈

ASJC Scopus subject areas

  • 電子、光磁材料
  • 原子與分子物理與光學
  • 凝聚態物理學

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