MOF@PVA beads for dynamic and low concentration VOC capture

Pamela Berilyn So; Chen Yu Liu; Yu Lun Lai; Cheng Shiuan Lee; Chia Her Lin

doi:10.1039/d2ma00257d

MOF@PVA beads for dynamic and low concentration VOC capture

Pamela Berilyn So, Chen Yu Liu, Yu Lun Lai, Cheng Shiuan Lee, Chia Her Lin^*

^*此作品的通信作者

化學系

研究成果: 雜誌貢獻 › 期刊論文 › 同行評審

1 引文斯高帕斯（Scopus）

摘要

This work explores the capacity of metal-organic framework (MOF)-polyvinyl alcohol (PVA) composites (MOF@PVA beads) in volatile organic compound (VOC) adsorption. The selected MOFs include HKUST-1, MIL-68, ZIF-8, A520, ZIF-67, and CAU-10, wherein the MOFs were optimized to be synthesized on a larger scale of production. Various proportions of the MOF@PVA bead composites were prepared to evaluate the optimal ratio to yield the best adsorption capacity. Most of the prepared MOF@PVA beads exhibited a higher VOC adsorption capacity as compared to commercially available activated carbon and zeolite adsorbents, proving the universality of the method of preparation. Among the composites, the MIL-68@PVA beads exhibited the best static VOC adsorption, while HKUST-1@PVA beads exhibited the best dynamic low concentration (200 ppm) toluene adsorption capacity.

原文	英語
期刊	Materials Advances
DOIs	https://doi.org/10.1039/d2ma00257d
出版狀態	接受/付印 - 2022

ASJC Scopus subject areas

化學（雜項）
材料科學(全部)

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10.1039/d2ma00257d

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@article{127694c5019d46078086f38c6ff5545b,

title = "MOF@PVA beads for dynamic and low concentration VOC capture",

abstract = "This work explores the capacity of metal-organic framework (MOF)-polyvinyl alcohol (PVA) composites (MOF@PVA beads) in volatile organic compound (VOC) adsorption. The selected MOFs include HKUST-1, MIL-68, ZIF-8, A520, ZIF-67, and CAU-10, wherein the MOFs were optimized to be synthesized on a larger scale of production. Various proportions of the MOF@PVA bead composites were prepared to evaluate the optimal ratio to yield the best adsorption capacity. Most of the prepared MOF@PVA beads exhibited a higher VOC adsorption capacity as compared to commercially available activated carbon and zeolite adsorbents, proving the universality of the method of preparation. Among the composites, the MIL-68@PVA beads exhibited the best static VOC adsorption, while HKUST-1@PVA beads exhibited the best dynamic low concentration (200 ppm) toluene adsorption capacity.",

author = "So, {Pamela Berilyn} and Liu, {Chen Yu} and Lai, {Yu Lun} and Lee, {Cheng Shiuan} and Lin, {Chia Her}",

note = "Funding Information: The authors would like to acknowledge the Taiwan Ministry of Science and Technology, for funding the research with grant numbers: MOST 110-2113-M-003-011-MY3 and MOST 110-2811-M-003-534. Publisher Copyright: {\textcopyright} 2022 The Author(s).",

year = "2022",

doi = "10.1039/d2ma00257d",

language = "English",

journal = "Materials Advances",

issn = "2633-5409",

publisher = "Royal Society of Chemistry",

}

TY - JOUR

T1 - MOF@PVA beads for dynamic and low concentration VOC capture

AU - So, Pamela Berilyn

AU - Liu, Chen Yu

AU - Lai, Yu Lun

AU - Lee, Cheng Shiuan

AU - Lin, Chia Her

N1 - Funding Information: The authors would like to acknowledge the Taiwan Ministry of Science and Technology, for funding the research with grant numbers: MOST 110-2113-M-003-011-MY3 and MOST 110-2811-M-003-534. Publisher Copyright: © 2022 The Author(s).

PY - 2022

Y1 - 2022

N2 - This work explores the capacity of metal-organic framework (MOF)-polyvinyl alcohol (PVA) composites (MOF@PVA beads) in volatile organic compound (VOC) adsorption. The selected MOFs include HKUST-1, MIL-68, ZIF-8, A520, ZIF-67, and CAU-10, wherein the MOFs were optimized to be synthesized on a larger scale of production. Various proportions of the MOF@PVA bead composites were prepared to evaluate the optimal ratio to yield the best adsorption capacity. Most of the prepared MOF@PVA beads exhibited a higher VOC adsorption capacity as compared to commercially available activated carbon and zeolite adsorbents, proving the universality of the method of preparation. Among the composites, the MIL-68@PVA beads exhibited the best static VOC adsorption, while HKUST-1@PVA beads exhibited the best dynamic low concentration (200 ppm) toluene adsorption capacity.

AB - This work explores the capacity of metal-organic framework (MOF)-polyvinyl alcohol (PVA) composites (MOF@PVA beads) in volatile organic compound (VOC) adsorption. The selected MOFs include HKUST-1, MIL-68, ZIF-8, A520, ZIF-67, and CAU-10, wherein the MOFs were optimized to be synthesized on a larger scale of production. Various proportions of the MOF@PVA bead composites were prepared to evaluate the optimal ratio to yield the best adsorption capacity. Most of the prepared MOF@PVA beads exhibited a higher VOC adsorption capacity as compared to commercially available activated carbon and zeolite adsorbents, proving the universality of the method of preparation. Among the composites, the MIL-68@PVA beads exhibited the best static VOC adsorption, while HKUST-1@PVA beads exhibited the best dynamic low concentration (200 ppm) toluene adsorption capacity.

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DO - 10.1039/d2ma00257d

M3 - Article

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JO - Materials Advances

JF - Materials Advances

SN - 2633-5409

ER -

MOF@PVA beads for dynamic and low concentration VOC capture

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