High-order nonlinear susceptibilities of helium

研究成果: 雜誌貢獻期刊論文同行評審

6 引文 斯高帕斯(Scopus)

摘要

With the goal of providing critically evaluated atomic data for modeling high harmonic generation processes in noble gases, we present calculations of frequency-dependent nonlinear susceptibilities of the ground state of helium, within the framework of Rayleigh-Schrödinger perturbation theory at lowest applicable order. The nonrelativistic, infinite-nuclear-mass, atomic Hamiltonian is decomposed in terms of Hylleraas coordinates and spherical harmonics, and the hierarchy of inhomogeneous equations of perturbation theory is solved iteratively. The mixed Hylleraas and Frankowski basis functions are employed to represent accurately the ground-state and perturbed wave functions. We believe our results for nonlinear susceptibilities of helium are the most accurate (and in many cases, the only) available to date, and they are offered as benchmark data for design of future multiphoton experiments.

原文英語
頁(從 - 到)4938-4945
頁數8
期刊Physical Review A - Atomic, Molecular, and Optical Physics
56
發行號6
DOIs
出版狀態已發佈 - 1997
對外發佈

ASJC Scopus subject areas

  • 原子與分子物理與光學

指紋

深入研究「High-order nonlinear susceptibilities of helium」主題。共同形成了獨特的指紋。

引用此