摘要
A-type antiferromagnetic (AF) order with a two-dimensional (2D) ferromagnetic short-range fluctuation was observed in the stoichiometric orthorhombic La1−xEuxMnO3+δ system (0 < x < 1, δ 0 with trivalent Mn3+). The observation of strong basal plane ferromagnetic coupling of the A-type AF order with fluctuation above antiferromagnetic Néel temperature TN strongly indicates a C-type orbital ordering of eg electrons at higher temperature throughout the whole system. Anomalous decrease of TN from 139 K for LaMnO3, to 91 K for La0.5Eu0.5MnO3 and down to 42 K for EuMnO3 is the result of weaker anisotropic superexchange interaction due to stronger Jahn-Teller lattice distortion in orbital-ordered EuMnO3 from power x-ray Rietveld analysis and Mn K-edge x-ray absorption near-edge structure spectroscopic study.
| 原文 | 英語 |
|---|---|
| 期刊 | Physical Review B - Condensed Matter and Materials Physics |
| 卷 | 67 |
| 發行號 | 21 |
| DOIs | |
| 出版狀態 | 已發佈 - 2003 6月 19 |
| 對外發佈 | 是 |
ASJC Scopus subject areas
- 電子、光磁材料
- 凝聚態物理學
指紋
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