Abstract
High-Tc superconducting YBa2Cu3Oy/ LaNiO3 (YBCO/LNO) bilayers were grown by off axis magnetron sputtering on (100) SrTiO3 substrates. Patterned samples with YBCO thicknesses of 50-100 nm and a fixed 20 nm LNO capping layer were measured with magnetic fields applied parallel to the c axis and within the ab plane. Relative to the well-studied single-layer YBCO, the bilayers exhibit a systematic suppression of superconductivity. Both the superconducting transition temperature (Tc) and the thermally activated flux-flow activation energy (U) decrease with decreasing YBCO thickness. The scaling of U(H) together with the temperature dependence of Hc2(T) near Tc is consistent with quasi-two-dimensional (2D) superconductivity confined at the YBCO/LNO interface. We attribute this behavior to interfacial strain- and redox-driven oxygen redistribution during LNO deposition, possibly accompanied by limited Ni intermixing, which together create a nanometer-scale region of reduced dimensionality and lower Tc. Interfacial superconductivity is established in oxide heterostructures and often shows quasi-2D behavior. Within this context, we present evidence consistent with quasi-2D behavior near Tc and discuss an interface-driven scenario in cuprate-nickelate bilayers. Given theoretical proposals that LaNiO3 heterostructures could host nontrivial band topology under suitable conditions, these results motivate further tests for possible topological superconductivity in this platform.
| Original language | English |
|---|---|
| Article number | 095015 |
| Journal | Superconductor Science and Technology |
| Volume | 38 |
| Issue number | 9 |
| DOIs | |
| Publication status | Published - 2025 Sept |
Keywords
- 2D-like superconductivity
- bilayer
- high-T YBCO
- sputtering
- topological superconductivity
ASJC Scopus subject areas
- Ceramics and Composites
- Condensed Matter Physics
- Metals and Alloys
- Electrical and Electronic Engineering
- Materials Chemistry
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