Room-Temperature Electrically Driven Tamm-Plasmon Exciton-Polariton LEDs Incorporating Monolayer Perovskite Quantum Dots

  • Meng Cheng Yen
  • , Wei Jie Hong
  • , Hsu Cheng Hsu
  • , Yuto Kajino
  • , Kaoru Tamada*
  • , Gong Ru Lin*
  • , Jinn Kong Sheu*
  • , Ya Ju Lee*
  • *Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

Abstract

Electrically driven exciton-polaritons in halide perovskites present a viable route toward room-temperature coherent light sources and polaritonic circuitry, yet experimental realizations remain limited. Here, we demonstrate a room-temperature, electrically driven exciton-polariton light-emitting diode (LED) by embedding a single monolayer of all-inorganic perovskite quantum dots (CsPbBr3 QDs) into a Tamm-plasmon (TP) microcavity comprising a distributed Bragg reflector (DBR) and a silver mirror. The subwavelength QD monolayer simultaneously provides strong exciton oscillator strength and reduces optical mode volume, yielding a large Rabi splitting of (Formula presented.). Time-resolved photoluminescence (PL) reveals a Purcell factor of (Formula presented.), evidencing accelerated radiative recombination and strengthened light-matter coupling. Under optical excitation, an accumulation of polariton population near the lower polariton branch minimum is observed, whereas momentum-resolved electroluminescence (EL) reveals a persistent polariton bottleneck effect under electrical injection. These results establish a scalable, fabrication-compatible platform for electrically driven polaritonic light sources at room temperature, advancing the development of integrated quantum photonic and optoelectronic technologies.

Original languageEnglish
JournalLaser and Photonics Reviews
DOIs
Publication statusAccepted/In press - 2025
Externally publishedYes

Keywords

  • CsPbBr quantum dots
  • exciton-polariton
  • polariton bottleneck effect
  • purcell factor
  • tamm plasmons

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Atomic and Molecular Physics, and Optics
  • Condensed Matter Physics

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