Resonant-enhanced dipolar interaction between THz-photons and confined acoustic phonons in nanostructures

  • Tzu Ming Liu*
  • , Ja Yu Lu
  • , Chung Chiu Kuo
  • , Meng Ju Yang
  • , Chih Wei Lai
  • , Pi Tai Chou
  • , Ming Hao Chang
  • , Hsiang Lin Liu
  • , Yu Tai Li
  • , Ci Ling Pan
  • , Shih Hung Lin
  • , Chieh Hsiung Kuan
  • , Chi Kuang Sun
  • *Corresponding author for this work

Research output: Chapter in Book/Report/Conference proceedingConference contribution

Abstract

By using a frequency-controlled narrow band THz source, a Fourier Transform Infrared (FTIR) spectroscopy system, and a frequency-controlled terahertz (THz) emitter, for the first time, we studied the THz photon absorption related to the THz confined acoustic vibrations in semiconductor nanocrystals. Through a specific charge separation in the CdSe/CdTe type-II nanocrystals and a piezoelectric coupling in the wurtzite CdSe nanocrystals, the THz photons can be resonantly coupled with (l=1) dipolar modes and the (l=0) breathing modes, respectively. Our results provide new mechanisms for low dimensional systems to convert a THz photon into a phonon of the same frequency..

Original languageEnglish
Title of host publicationUltrafast Phenomena in Semiconductors and Nanostructure Materials XII
DOIs
Publication statusPublished - 2008
EventUltrafast Phenomena in Semiconductors and Nanostructure Materials XII - San Jose, CA, United States
Duration: 2008 Jan 202008 Jan 23

Publication series

NameProceedings of SPIE - The International Society for Optical Engineering
Volume6892
ISSN (Print)0277-786X

Conference

ConferenceUltrafast Phenomena in Semiconductors and Nanostructure Materials XII
Country/TerritoryUnited States
CitySan Jose, CA
Period2008/01/202008/01/23

Keywords

  • Confined acoustic phonons
  • Piezoelectric nanocrystals
  • Terahertz
  • Type-II nanocrystals

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics
  • Computer Science Applications
  • Applied Mathematics
  • Electrical and Electronic Engineering

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