Low-Threshold Lasing from 2D Homologous Organic-Inorganic Hybrid Ruddlesden-Popper Perovskite Single Crystals

Chinnambedu Murugesan Raghavan, Tzu Pei Chen, Shao Sian Li*, Wei Liang Chen, Chao Yuan Lo, Yu Ming Liao, Golam Haider, Cheng Chieh Lin, Chia Chun Chen, Raman Sankar, Yu Ming Chang, Fang Cheng Chou, Chun Wei Chen

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

174 Citations (Scopus)

Abstract

Organic-inorganic hybrid two-dimensional (2D) perovskites have recently attracted great attention in optical and optoelectronic applications due to their inherent natural quantum-well structure. We report the growth of high-quality millimeter-sized single crystals belonging to homologous two-dimensional (2D) hybrid organic-inorganic Ruddelsden-Popper perovskites (RPPs) of (BA)2(MA)-rfnet-1PbnI3n+1 (n = 1, 2, and 3) by a slow evaporation at a constant-temperature (SECT) solution-growth strategy. The as-grown 2D hybrid perovskite single crystals exhibit excellent crystallinity, phase purity, and spectral uniformity. Low-threshold lasing behaviors with different emission wavelengths at room temperature have been observed from the homologous 2D hybrid RPP single crystals. Our result demonstrates that solution-growth homologous organic-inorganic hybrid 2D perovskite single crystals open up a new window as a promising candidate for optical gain media.

Original languageEnglish
Pages (from-to)3221-3228
Number of pages8
JournalNano Letters
Volume18
Issue number5
DOIs
Publication statusPublished - 2018 May 9

Keywords

  • 2D RPP single crystals
  • lasing
  • photoluminescence
  • solution growth

ASJC Scopus subject areas

  • Bioengineering
  • General Chemistry
  • General Materials Science
  • Condensed Matter Physics
  • Mechanical Engineering

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