Enhancing UV-emissions through optical and electronic dual-function tuning of Ag nanoparticles hybridized with n-ZnO nanorods/p-GaN heterojunction light-emitting diodes

Yung Chi Yao, Zu Po Yang, Jung Min Hwang, Yi Lun Chuang, Chia Ching Lin, Jing Yu Haung, Chun Yang Chou, Jinn Kong Sheu, Meng Tsan Tsai, Ya Ju Lee

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18 Citations (Scopus)

Abstract

ZnO nanorods (NRs) and Ag nanoparticles (NPs) are known to enhance the luminescence of light-emitting diodes (LEDs) through the high directionality of waveguide mode transmission and efficient energy transfer of localized surface plasmon (LSP) resonances, respectively. In this work, we have demonstrated Ag NP-incorporated n-ZnO NRs/p-GaN heterojunctions by facilely hydrothermally growing ZnO NRs on Ag NP-covered GaN, in which the Ag NPs were introduced and randomly distributed on the p-GaN surface to excite the LSP resonances. Compared with the reference LED, the light-output power of the near-band-edge (NBE) emission (ZnO, λ = 380 nm) of our hybridized structure is increased almost 1.5-2 times and can be further modified in a controlled manner by varying the surface morphology of the surrounding medium of the Ag NPs. The improved light-output power is mainly attributed to the LSP resonance between the NBE emission of ZnO NRs and LSPs in Ag NPs. We also observed different behaviors in the electroluminescence (EL) spectra as the injection current increases for the treatment and reference LEDs. This observation might be attributed to the modification of the energy band diagram for introducing Ag NPs at the interface between n-ZnO NRs and p-GaN. Our results pave the way for developing advanced nanostructured LED devices with high luminescence efficiency in the UV emission regime.

Original languageEnglish
Pages (from-to)4463-4474
Number of pages12
JournalNanoscale
Volume8
Issue number8
DOIs
Publication statusPublished - 2016 Feb 28

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Nanorods
Light emitting diodes
Heterojunctions
Tuning
Nanoparticles
Surface plasmon resonance
Luminescence
Electroluminescence
Band structure
Energy transfer
Surface morphology
Waveguides

ASJC Scopus subject areas

  • Materials Science(all)

Cite this

Enhancing UV-emissions through optical and electronic dual-function tuning of Ag nanoparticles hybridized with n-ZnO nanorods/p-GaN heterojunction light-emitting diodes. / Yao, Yung Chi; Yang, Zu Po; Hwang, Jung Min; Chuang, Yi Lun; Lin, Chia Ching; Haung, Jing Yu; Chou, Chun Yang; Sheu, Jinn Kong; Tsai, Meng Tsan; Lee, Ya Ju.

In: Nanoscale, Vol. 8, No. 8, 28.02.2016, p. 4463-4474.

Research output: Contribution to journalArticle

Yao, Yung Chi ; Yang, Zu Po ; Hwang, Jung Min ; Chuang, Yi Lun ; Lin, Chia Ching ; Haung, Jing Yu ; Chou, Chun Yang ; Sheu, Jinn Kong ; Tsai, Meng Tsan ; Lee, Ya Ju. / Enhancing UV-emissions through optical and electronic dual-function tuning of Ag nanoparticles hybridized with n-ZnO nanorods/p-GaN heterojunction light-emitting diodes. In: Nanoscale. 2016 ; Vol. 8, No. 8. pp. 4463-4474.
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