Anomalous variation of A-type antiferromagnetic order and two-dimensional ferromagnetic fluctuation in orbital-ordered La1−xEuxMnO3

C. T. Chen; B. N. Lin; Y. Y. Hsu; J. D. Liao; W. H. Cheng; C. Y. Lin; H. C. Ku; J. F. Lee; L. Y. Jang; D. G. Liu

doi:10.1103/PhysRevB.67.214424

Anomalous variation of A-type antiferromagnetic order and two-dimensional ferromagnetic fluctuation in orbital-ordered La_1−xEu_xMnO₃

C. T. Chen, B. N. Lin, Y. Y. Hsu, J. D. Liao, W. H. Cheng, C. Y. Lin, H. C. Ku, J. F. Lee, L. Y. Jang, D. G. Liu

Research output: Contribution to journal › Article › peer-review

18 Citations (Scopus)

Abstract

A-type antiferromagnetic (AF) order with a two-dimensional (2D) ferromagnetic short-range fluctuation was observed in the stoichiometric orthorhombic La_1−xEu_xMnO_3+δ system (0 < x < 1, δ 0 with trivalent Mn³⁺). The observation of strong basal plane ferromagnetic coupling of the A-type AF order with fluctuation above antiferromagnetic Néel temperature T_N strongly indicates a C-type orbital ordering of e_g electrons at higher temperature throughout the whole system. Anomalous decrease of T_N from 139 K for LaMnO₃, to 91 K for La_0.5Eu_0.5MnO₃ and down to 42 K for EuMnO₃ is the result of weaker anisotropic superexchange interaction due to stronger Jahn-Teller lattice distortion in orbital-ordered EuMnO₃ from power x-ray Rietveld analysis and Mn K-edge x-ray absorption near-edge structure spectroscopic study.

Original language	English
Journal	Physical Review B - Condensed Matter and Materials Physics
Volume	67
Issue number	21
DOIs	https://doi.org/10.1103/PhysRevB.67.214424
Publication status	Published - 2003 Jun 19
Externally published	Yes

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Condensed Matter Physics

Access to Document

10.1103/PhysRevB.67.214424

Cite this

Chen, C. T., Lin, B. N., Hsu, Y. Y., Liao, J. D., Cheng, W. H., Lin, C. Y., Ku, H. C., Lee, J. F., Jang, L. Y., & Liu, D. G. (2003). Anomalous variation of A-type antiferromagnetic order and two-dimensional ferromagnetic fluctuation in orbital-ordered La_1−xEu_xMnO₃. Physical Review B - Condensed Matter and Materials Physics, 67(21). https://doi.org/10.1103/PhysRevB.67.214424

@article{e32a2828176f4d5cb6ad834c051ab929,

title = "Anomalous variation of A-type antiferromagnetic order and two-dimensional ferromagnetic fluctuation in orbital-ordered La1−xEuxMnO3",

abstract = "A-type antiferromagnetic (AF) order with a two-dimensional (2D) ferromagnetic short-range fluctuation was observed in the stoichiometric orthorhombic La1−xEuxMnO3+δ system (0 < x < 1, δ 0 with trivalent Mn3+). The observation of strong basal plane ferromagnetic coupling of the A-type AF order with fluctuation above antiferromagnetic N{\'e}el temperature TN strongly indicates a C-type orbital ordering of eg electrons at higher temperature throughout the whole system. Anomalous decrease of TN from 139 K for LaMnO3, to 91 K for La0.5Eu0.5MnO3 and down to 42 K for EuMnO3 is the result of weaker anisotropic superexchange interaction due to stronger Jahn-Teller lattice distortion in orbital-ordered EuMnO3 from power x-ray Rietveld analysis and Mn K-edge x-ray absorption near-edge structure spectroscopic study.",

author = "Chen, {C. T.} and Lin, {B. N.} and Hsu, {Y. Y.} and Liao, {J. D.} and Cheng, {W. H.} and Lin, {C. Y.} and Ku, {H. C.} and Lee, {J. F.} and Jang, {L. Y.} and Liu, {D. G.}",

year = "2003",

month = jun,

day = "19",

doi = "10.1103/PhysRevB.67.214424",

language = "English",

volume = "67",

journal = "Physical Review B - Condensed Matter and Materials Physics",

issn = "1098-0121",

publisher = "American Physical Society",

number = "21",

}

TY - JOUR

T1 - Anomalous variation of A-type antiferromagnetic order and two-dimensional ferromagnetic fluctuation in orbital-ordered La1−xEuxMnO3

AU - Chen, C. T.

AU - Lin, B. N.

AU - Hsu, Y. Y.

AU - Liao, J. D.

AU - Cheng, W. H.

AU - Lin, C. Y.

AU - Ku, H. C.

AU - Lee, J. F.

AU - Jang, L. Y.

AU - Liu, D. G.

PY - 2003/6/19

Y1 - 2003/6/19

N2 - A-type antiferromagnetic (AF) order with a two-dimensional (2D) ferromagnetic short-range fluctuation was observed in the stoichiometric orthorhombic La1−xEuxMnO3+δ system (0 < x < 1, δ 0 with trivalent Mn3+). The observation of strong basal plane ferromagnetic coupling of the A-type AF order with fluctuation above antiferromagnetic Néel temperature TN strongly indicates a C-type orbital ordering of eg electrons at higher temperature throughout the whole system. Anomalous decrease of TN from 139 K for LaMnO3, to 91 K for La0.5Eu0.5MnO3 and down to 42 K for EuMnO3 is the result of weaker anisotropic superexchange interaction due to stronger Jahn-Teller lattice distortion in orbital-ordered EuMnO3 from power x-ray Rietveld analysis and Mn K-edge x-ray absorption near-edge structure spectroscopic study.

AB - A-type antiferromagnetic (AF) order with a two-dimensional (2D) ferromagnetic short-range fluctuation was observed in the stoichiometric orthorhombic La1−xEuxMnO3+δ system (0 < x < 1, δ 0 with trivalent Mn3+). The observation of strong basal plane ferromagnetic coupling of the A-type AF order with fluctuation above antiferromagnetic Néel temperature TN strongly indicates a C-type orbital ordering of eg electrons at higher temperature throughout the whole system. Anomalous decrease of TN from 139 K for LaMnO3, to 91 K for La0.5Eu0.5MnO3 and down to 42 K for EuMnO3 is the result of weaker anisotropic superexchange interaction due to stronger Jahn-Teller lattice distortion in orbital-ordered EuMnO3 from power x-ray Rietveld analysis and Mn K-edge x-ray absorption near-edge structure spectroscopic study.

UR - http://www.scopus.com/inward/record.url?scp=84872738122&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=84872738122&partnerID=8YFLogxK

U2 - 10.1103/PhysRevB.67.214424

DO - 10.1103/PhysRevB.67.214424

M3 - Article

AN - SCOPUS:84872738122

SN - 1098-0121

VL - 67

JO - Physical Review B - Condensed Matter and Materials Physics

JF - Physical Review B - Condensed Matter and Materials Physics

IS - 21

ER -

Anomalous variation of A-type antiferromagnetic order and two-dimensional ferromagnetic fluctuation in orbital-ordered La_1−xEu_xMnO₃

Abstract

ASJC Scopus subject areas

Access to Document

Other files and links

Fingerprint

Cite this